Chemistry

Electron spin resonance in a strong-rung spin- 12 Heisenberg ladder

A. N. Ponomaryov, HZDR - Helmholtz-Zentrum Dresden-Rossendorf
M. Ozerov, HZDR - Helmholtz-Zentrum Dresden-Rossendorf
L. Zviagina, HZDR - Helmholtz-Zentrum Dresden-Rossendorf
J. Wosnitza, HZDR - Helmholtz-Zentrum Dresden-Rossendorf
K. Y. Povarov, ETH Zürich
F. Xiao, ETH Zürich
A. Zheludev, ETH Zürich
C. Landee, Clark University
E. ČiŽmár, Pavol Jozef Šafárik University in Košice
A. A. Zvyagin, Max Planck Institute for the Physics of Complex Systems
S. A. Zvyagin, HZDR - Helmholtz-Zentrum Dresden-Rossendorf

Abstract

Cu(C8H6N2)Cl2, a strong-rung spin-12 Heisenberg ladder compound, is probed by means of electron spin resonance (ESR) spectroscopy in the field-induced gapless phase above Hc1. The temperature dependence of the ESR linewidth is analyzed in the quantum field theory framework, suggesting that the anisotropy of magnetic interactions plays a crucial role, determining the peculiar low-temperature ESR linewidth behavior. In particular, it is argued that the uniform Dzyaloshinskii-Moriya interaction (which is allowed on the bonds along the ladder legs) can be the source of this behavior in Cu(C8H6N2)Cl2.